ajoknoblauch
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Having a copy of your previous crossing document is kind of a difficult task if it is the first time you are entering Argentina with your car. Based on my experience with Chilean customs at Libertadores I would avoid that crossing and drive accross Pehuenche (a little south of Libertadores). Or if you driving to Bariloche then you could just cross at Cardenal Samoré. At both I had no issues with my Chilean car.
If you want to go to Mendoza City, Pehuenche is a pretty major detour, some 363 km southeast of Santiago. It's another 72 km to the Argentine border post at Las Loicas, from which it's several hundred km more to Mendoza. That said, it's a very scenic route, but I only do it if I have specific reason to cross there.